Features of plasmonic enhancement of luminescence of molecular aggregates of cyanine dyes
Abstract
The article examines the effect of plasmon resonance of gold nanoparticles on the luminescent properties of molecular aggregates (J-aggregates) of two cyanine dyes, PIC and TDBC. It is shown that the luminescence enhancement of J-aggregates due to the exciton-plasmon interaction occurs in a very similar manner for both types of aggregates, namely: the largest enhancement factor is achieved at a distance between J-aggregates and nanoparticles of 15-20 nm, while the exciton delocalization length increases and increasing their lifetime, as well as suppressing the process of exciton self-trapping. However, these effects are more pronounced for PIC J-aggregates than for TDBC J-aggregates, despite the latter exhibiting better excitonic characteristics. It is proposed that the main factor of the detected discrepancies is the different structure of the exciton bands for J-aggregates and, accordingly, the different degree of overlap of their absorption bands with the plasmon resonance band of gold nanoparticles.
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