The influence of defects and impurity atoms on the physical and mechanical properties of nanostructured coatings in the boundary region separating them
Keywords:
nanostructured coatings, phase and elemental composition, adhesion, superhardness, defects, segregation, stress
Abstract
Using unique methods: positron annihilation, proton microbeam, Rutherford backscattering (RBS) of ions, microprobe using EDSX with SEM, X-ray diffraction (XRD), X-ray strain measurement (α-sin2ψ), tests of nanohardness, elastic modulus, index plasticity and scratch tests were investigated nanostructured coatings Ti-Si-N; Ti-Hf-Si-N; (Ti-Hf-Zr-V-Nb)N, grown by cathodic vacuum arc source. Defects’ profiles were obtained at all depth of coating, and effect of thermal annealing at 600 °C (30 min) on the change of the defect structure, elastic-directed state, the phase composition and the redistribution of impurity atoms as a result of thermal diffusion and segregation processes boundaries and sub-boundaries of nanograins were studied. An increase of hardness after annealing, decreasing of the elastic-strain state, the redistribution of impurity atoms and defects were observed.
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References
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Sobol’ O.V., Andreev A.A., Gorban’ V.F., Krapivka N.A., Stolbovoj V.A., Serdyuk I.V., Fil’chikov V.E. O vosproizvodimosti odnofaznogo strukturnogo sostoyaniya mnogo‘elementnoj vysoko‘entropijnoj sistemy Ti-V-Zr-Nb-Hf i vysokotverdyh nitridov na ee osnove pri ih formirovanii vakuumnodugovym metodom//Pis’ma v ZhTF. – 2012. – T. 38, Vyp. 13. – S. 41-48.
Pogrebnyak A.D., Shpak A.P., Azarenkov N.A., Beresnev V.M. Struktura i svojstva tverdyh i sverhtverdyh nanokompozitnyh pokrytij//UFN. – 2009. – T. 179. – S. 35-64.
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Pogrebnyak A.D., Sobol’ O.V., Beresnev V.M. Osobennosti strukturnogo sostoyaniya i mehanicheskih svojstv pokrytij ZrN i Zr (Ti) -Si-N, poluchennyh ionno-plazmennymi metodami//Pis’ma v ZhTF. – 2009. – T. 35. – S. 103-110.
Pogrebnjak A.D., Ponomarev A.G., Shpak A.P., Kunitskii Yu.A. Application of micro- and nanoprobes to the analysis of small-sized 3D materials, nanosystems, and nanoobjects//Physics-Uspekhi. – 2012. – Vol. 55. – P. 270-300.
Musil J. Hard and superhard nanocomposite coatings//Surface and Coatings Technology. – 2000. – Vol. 125. – P. 322-330.
Korotaev A.D., Borisov V.D., Moshkov V.Yu. Uprugo-napryazhennoe sostoyanie mnogo‘elementnyh sverhtverdyh pokrytij//Fizicheskaya mezomehanika. – 2009. – T. 12, № 4. – S. 79-91.
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Andrievskij R.A., Kalinnikov G.V., Hellgren N., Sandstrorm P., Shtanskij D.V. Nanoindentirovanie i deformacionnye harakteristiki nanostrukturnyh boridonitridnyh plenok//FTT. – 2000. – T. 42, № 9. – P. 1624-1627.
Andrievskij R.A., Glezer A.M. Prochnost’ nanostruktur//UFN.– 2009.– T. 179, № 4. – S. 337-358.
Zhang R.F., Argon A.S., Veprek S. Electronic structure, stability, and mechanism of the decohesion and
shear of interfaces in superhard nanocomposites and heterostructures//Phys. Rew. – 2009. – Vol. 79. – P. 245426.
Musil J., Baroch P., Zeman P. Hard nanocomposite coatings. Present Status and Trends: in Book Plasma Surface Engineering and its Practical Applications/ Edit. R. Wei, Research Singpost. Publ, 2007.
Uglov V.V., Anischik V.M., Zlotskij S.V., Abadias G., Dub. S.N. Structural and mechanical stability upon annealing of arc-deposited Ti-Zr-N coatings// Surf. and Coat. Tech. – 2008. – Vol. 202. – P. 2394-2398.
Shaefer H.-E. Investigation of Thermal Equilibrium Vacancies in Metals by Positron Annihilation//Phys. Stat. Sol. (a). – 1987. – Vol. 102, Iss. 1. – P. 47-65.
Rempel’ S.V., Gusev A.I. Poverhnostnaya segregaciya v raspadayuschihsya karbidnyh tverdyh rastvorah//Pis’ma v Zh‘ETF, 2008. – T. 88, Vyp. 7. – S. 508-513.
Whschum R., Farber P., Dittmar R., Scharwaechter P., Frank W., Schaefer H.-E. Thermal Vacancy Formation and Self-Diffusion in Intermetallic Fe3Si Nanocrystallites of Nanocomposite Alloys//Phys. Rev. Lett. 1997. – Vol. 79, Iss. 24. – P. 4918-4921.
Lavrent’ev V.I., Pogrebnyak A.D., R. Shandrik, Lokal’nye poverhnostnye segregacii implantirovannogo alyuminiya v slabodefektnom kristalle zheleza//Pis’ma v Zh‘ETF. – 1997. – T. 65, Vyp. 1.– S. 86-89.
Gusev A.I. Nanomaterialy, nanostruktury, nanotehnologii. – M.: FIZMATLIT, 2005. – 416 c.
Veprek S., Veprek-Heijman M.G.J. Limits to the preperation os superhard nanocomposites: Impurities, deposition and annealing temperature//Thin Solid Films. – 2012. – Vol. 522, – P. 274-282.
Krause-Rehberg R. and Leipner H.S. Positron Annihilation on Semiconductors. Stude of Defects// Springer-Verlag, Berlin. Series “Solid-State Sciences”. – 1999. – Vol. 127. – P. 378.
Pogrebnjak A.D., Shpak A.P., Beresnev V.M., Kolesnikov D.A., Kunitsky Y u.A., Sobol O.V., Uglov V.V., Komarov F.F., Shypylenko A.P., Demyanenko A.A., Baidak V.S., Grudnitskii V.V. Effect of Thermal Annealing in Vacuum and Air on Nanograin Sizes in Hard and Superhard Coatings Zr-TiSi-N Journal of Nanoscience and Nanotechnology. – 2012. – Vol. 12, №12. - P. 9213-9219.
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Korotaev A.D., Borisov D.P., Meshkov V.Yu., Ovchinnikov S.V. i dr. Nanokompozitnye i nanostrukturnye sverhtverdye pokrytiya sistemy Ti-Si-B-N// Izv. Vuzov. Fizika. – 2007. – T. 50, № 10. – C. 13-23.
Korotaev A.D., Borisov V.D., Moshkov V.Yu., Ovchinnikov C.V., Pinzhin Yu.P., Tyumencev A.N. Uprugonapryazhennoe sostoyanie mnogo‘elementnyh sverhtverdyh pokrytij//Fizicheskaya mezomehanika. – 2009. – T. 12, № 4. – S. 79-92.
Musil J. Hard nanocomposite coatings: Thermal stability, oxidation resistance and toughness//Surf. and Coat. Tech. – 2012. – Vol. 207. – P. 50-65.
Misaelides P., Hadzidimitrion A., Noli F., Pavlidou E., Pogrebnjak A.D.//Appl. Surf. Sci. – 2006. – Vol. 252 (23). – P. 8043-8049.
Pogrebnyak A.D., Ponomarev A.G., Shpak A.P., Kunickij Yu.A. Primenenie mikro- i nanozondov dlya analiza malorazmernyh 3D materialov, nanosistem i nanoob‘ektov//UFN. – 2012. – T. 182, № 3. – S. 287-321.
Pogrebnyak A.D., Beresnev V.M., Dem’yanenko A.A., Bajdak V.S, Komarov F.F., Kaverin M.V., Mahmudov N. and Kolesnikov D.A. Adgezionnaya prochnost’ i sverhtverdost’, fazovyj i ‘elementnyj sostav nanostrukturnyh pokrytij, sformirovannyh na osnove Ti-Hf-Si-N//FTT. – 2012. – T. 54, № 9. – S. 1882-1890.
Pogrebnyak A.D., Sobol’ O.V., Beresnev V.M., Turbin P.V., Dub S.N., Kirik G.V., Dmitrenko A.E. Osobennosti strukturnogo sostoyaniya i mehanicheskih svojstv pokrytij ZrN i Zr(Ti)-Si-N, poluchennyh ionno-plazmennymi metodami//Pis’ma v ZhTF. – 2009. – T. 35, № 19. – S. 103-110.
Dolique V., Thomann A.-L., Brault P., Tessier Y., Gillon P. Complex structure/composition relationship in thin films of AlCoCrCuFeNi high entropy alloy// Materials Chemistry and Physics. – 2009. – Vol. 117, № 1. – Р. 142-147.
Tsai M., Wang C., Tsai C., Shen W., Yeh J., Gan J., Wu W. Thermal Stability and Performance of NbSiTaTiZr High-Entropy Alloy Barrier for Copper Metallization//Electrochemical Society. – 2011. – Vol. 158, № 11. – P. H1161-H1165.
Li A., Zhang X. Acta Metallurgica Sinica//English Letters. – 2009. – Vol. 22, № 3. – P. 219-224.
Firstov S.A., Gorban’ V.F., Krapivka N.A., Pechkovskij ‘E.P. Uprochnenie i mehanicheskie svojstva lityh vysoko‘entropijnyh splavov//Kompozity i nanoctruktury. – 2011. – № 2. – S. 5-20.
Pogrebnjak, A.D. Uglov, V.V. Il’yashenko, M.V. Beresnev, V.M. Shpak, A.P. Kaverin, M.V. Erdybaeva, N.K. Kunitskyi, Yu.A. Tyurin, Yu.N. Kolisnichenko, O.V. Makhmudov, N.A. Shypylenko, A.P. Nano-Microcomposite and Combined Coatings on Ti-Si-NAA/C-Co-Cr/Steel and Ti-Si-N/(Cr3C2)75(NiCr)25 Base: Their Structure and Properties//Ceramic Engineering and Science Proceedings, Wiley. – 2010. – Vol. 31, № 7. – P. 115-126.
Sobol’ O.V., Pogrebnyak A.D., Beresnev V.M. Vli-yanie uslovij polucheniya na fazovyj sostav, strukturu i mehanicheskie harakteristiki vakuumnodugovyh pokrytij sistemy Zr-Ti-Si-N//FMM. – 2011. – T. 112, № 2. – S. 199-206.
Musil J., Vlcek J. and Zeman P.. Hard amorphous nanocomposite coatings with oxidation resistance above 1000 °C//Advances in Applied Ceramics. – 2008. – Vol. 107, № 3. – P. 148-154.
Azarenkov N.A., Sobol’ O.V., Beresnev V.M., Pogrebnyak O.D., Litovchenko S.V., Ivanov O.N. Materialovedenie neravnovesnogo sostoyaniya modificirovannoj poverhnosti: monografiya. – Sumy: Sumskij gosudarstvennyj universitet, 2012. – 683 c.
Azarenkov N.A., Beresnev V.M., Pogrebnyak A.D., Kolesnikov D.A. Nanostrukturnye pokrytiya i nanomaterialy: Osnovy polucheniya. Svojstva. Oblasti primeneniya: Osobennosti sovremennogo nanostrukturnogo napravleniya v nanotehnologii. – M.: URSS, 2012. – 368 c.
Lavrent’ev V.I., Pogrebnyak A.D., Shandrik R. ‘Evolyuciya vakansionnyh defektov v poverhnostnyh sloyah metalla pri impul’snom vozdejstvii ‘elektronnym puchkom//Pis’ma v Zh‘ETF. – 1997. – № 65. – C. 618-622.
Rempel’ S.V., Gusev A.I. Poverhnostnaya segregaciya v raspadayuschihsya karbidnyh tverdyh rastvorah//Pis’ma v Zh‘ETF. – 2008. № 88.– S. 508-513.
Simnra.com.
Pogrebnyak A.D., Ponomarev A.G., Kolesnikov D.A., Beresnev V.M., Komarov F.F., Mel’nik S.S., Kaverin M.V. Effect of mass transfer and segregation on the formation of superhard nanostructured Ti-Hf-N(Fe) coatings//Technical Physics Letters. – 2012. – Vol. 38, No. 7. – P. 623-626.
Krause-Rehberg R., Leipner H.S. Positron Annihilation in Semiconductors: Defect Studies. – New York: Springer-Verlag Berlin Heidelberg, 2003. – P. 387.
Pogrebnjak A.D., Il’yashenko M.V., Kaverin M.V., Shypylenko A.P., Pshyk A.V., Beresnev V.M., Kirik G.V., Erdybayeva N.K., Makhmudov N.A., Kolisnichenko O.V., Tyurin Yu.N., Shpak A.P. Physical and mechanical properties of the nanocomposite and combined Ti-N-Si/WC-Co-Cr/ and Ti-N-Si/ (Cr3C2)75-(NiCr)25 coatings//Journal of Nano- and Electronic Physics. – 2009. – Vol. 1. – P. 66-77.
Sobol’ O.V., Pogrebnyak A.D., Beresnev V.M. Vliyanie uslovij polucheniya na fazovyj sostav, strukturu i mehanicheskie harakteristiki vakuumno-dugovyh pokrytij sistemy Zr-Ti-Si-N//FMM. – 2011. – T. 112, №2. – S.199-206.
Sobol’ O.V., Andreev A.A., Gorban’ V.F., Krapivka N.A., Stolbovoj V.A., Serdyuk I.V., Fil’chikov V.E. O vosproizvodimosti odnofaznogo strukturnogo sostoyaniya mnogo‘elementnoj vysoko‘entropijnoj sistemy Ti-V-Zr-Nb-Hf i vysokotverdyh nitridov na ee osnove pri ih formirovanii vakuumnodugovym metodom//Pis’ma v ZhTF. – 2012. – T. 38, Vyp. 13. – S. 41-48.
Pogrebnyak A.D., Shpak A.P., Azarenkov N.A., Beresnev V.M. Struktura i svojstva tverdyh i sverhtverdyh nanokompozitnyh pokrytij//UFN. – 2009. – T. 179. – S. 35-64.
Smitlz K. Dzh. Metally: sprav. Izdan./Per. s angl. Spravochnik. Izdanie 5-e, 1980. − 447 c.
Pogrebnyak A.D., Sobol’ O.V., Beresnev V.M. Osobennosti strukturnogo sostoyaniya i mehanicheskih svojstv pokrytij ZrN i Zr (Ti) -Si-N, poluchennyh ionno-plazmennymi metodami//Pis’ma v ZhTF. – 2009. – T. 35. – S. 103-110.
Pogrebnjak A.D., Ponomarev A.G., Shpak A.P., Kunitskii Yu.A. Application of micro- and nanoprobes to the analysis of small-sized 3D materials, nanosystems, and nanoobjects//Physics-Uspekhi. – 2012. – Vol. 55. – P. 270-300.
Musil J. Hard and superhard nanocomposite coatings//Surface and Coatings Technology. – 2000. – Vol. 125. – P. 322-330.
Korotaev A.D., Borisov V.D., Moshkov V.Yu. Uprugo-napryazhennoe sostoyanie mnogo‘elementnyh sverhtverdyh pokrytij//Fizicheskaya mezomehanika. – 2009. – T. 12, № 4. – S. 79-91.
Andrievskij R.A., Kalinnikov G.V., Hellgren N., Sandstrorm P., Shtanskij D.V. Nanoindentirovanie i deformacionnye harakteristiki nanostrukturnyh boridonitridnyh plenok//FTT. – 2000. – T. 42, № 9. – P. 1624-1627.
Andrievskij R.A., Glezer A.M. Prochnost’ nanostruktur//UFN.– 2009.– T. 179, № 4. – S. 337-358.
Zhang R.F., Argon A.S., Veprek S. Electronic structure, stability, and mechanism of the decohesion and
shear of interfaces in superhard nanocomposites and heterostructures//Phys. Rew. – 2009. – Vol. 79. – P. 245426.
Musil J., Baroch P., Zeman P. Hard nanocomposite coatings. Present Status and Trends: in Book Plasma Surface Engineering and its Practical Applications/ Edit. R. Wei, Research Singpost. Publ, 2007.
Uglov V.V., Anischik V.M., Zlotskij S.V., Abadias G., Dub. S.N. Structural and mechanical stability upon annealing of arc-deposited Ti-Zr-N coatings// Surf. and Coat. Tech. – 2008. – Vol. 202. – P. 2394-2398.
Shaefer H.-E. Investigation of Thermal Equilibrium Vacancies in Metals by Positron Annihilation//Phys. Stat. Sol. (a). – 1987. – Vol. 102, Iss. 1. – P. 47-65.
Rempel’ S.V., Gusev A.I. Poverhnostnaya segregaciya v raspadayuschihsya karbidnyh tverdyh rastvorah//Pis’ma v Zh‘ETF, 2008. – T. 88, Vyp. 7. – S. 508-513.
Whschum R., Farber P., Dittmar R., Scharwaechter P., Frank W., Schaefer H.-E. Thermal Vacancy Formation and Self-Diffusion in Intermetallic Fe3Si Nanocrystallites of Nanocomposite Alloys//Phys. Rev. Lett. 1997. – Vol. 79, Iss. 24. – P. 4918-4921.
Lavrent’ev V.I., Pogrebnyak A.D., R. Shandrik, Lokal’nye poverhnostnye segregacii implantirovannogo alyuminiya v slabodefektnom kristalle zheleza//Pis’ma v Zh‘ETF. – 1997. – T. 65, Vyp. 1.– S. 86-89.
Gusev A.I. Nanomaterialy, nanostruktury, nanotehnologii. – M.: FIZMATLIT, 2005. – 416 c.
Veprek S., Veprek-Heijman M.G.J. Limits to the preperation os superhard nanocomposites: Impurities, deposition and annealing temperature//Thin Solid Films. – 2012. – Vol. 522, – P. 274-282.
Krause-Rehberg R. and Leipner H.S. Positron Annihilation on Semiconductors. Stude of Defects// Springer-Verlag, Berlin. Series “Solid-State Sciences”. – 1999. – Vol. 127. – P. 378.
Pogrebnjak A.D., Shpak A.P., Beresnev V.M., Kolesnikov D.A., Kunitsky Y u.A., Sobol O.V., Uglov V.V., Komarov F.F., Shypylenko A.P., Demyanenko A.A., Baidak V.S., Grudnitskii V.V. Effect of Thermal Annealing in Vacuum and Air on Nanograin Sizes in Hard and Superhard Coatings Zr-TiSi-N Journal of Nanoscience and Nanotechnology. – 2012. – Vol. 12, №12. - P. 9213-9219.
Pogrebnjak A.D., Beresnev V.M. Nanocoatings Nanosystems Nanotechnologies, Bentham//Sci. Publ., Bentham e books. – 2012. – P. 158.
Korotaev A.D., Borisov D.P., Meshkov V.Yu., Ovchinnikov S.V. i dr. Nanokompozitnye i nanostrukturnye sverhtverdye pokrytiya sistemy Ti-Si-B-N// Izv. Vuzov. Fizika. – 2007. – T. 50, № 10. – C. 13-23.
Korotaev A.D., Borisov V.D., Moshkov V.Yu., Ovchinnikov C.V., Pinzhin Yu.P., Tyumencev A.N. Uprugonapryazhennoe sostoyanie mnogo‘elementnyh sverhtverdyh pokrytij//Fizicheskaya mezomehanika. – 2009. – T. 12, № 4. – S. 79-92.
Musil J. Hard nanocomposite coatings: Thermal stability, oxidation resistance and toughness//Surf. and Coat. Tech. – 2012. – Vol. 207. – P. 50-65.
Misaelides P., Hadzidimitrion A., Noli F., Pavlidou E., Pogrebnjak A.D.//Appl. Surf. Sci. – 2006. – Vol. 252 (23). – P. 8043-8049.
Published
2017-07-28
How to Cite
Каверин, М. В., Krause-Rehberg, R., Береснев, В. М., Постольный, Б. А., Колесников, Д. А., Якущенко, И. В., Билокур, М. А., & Жоллыбеков, Б. Р. (2017). The influence of defects and impurity atoms on the physical and mechanical properties of nanostructured coatings in the boundary region separating them. Journal of Surface Physics and Engineering, 11(2), 160 - 184. Retrieved from https://periodicals.karazin.ua/pse/article/view/8768
Section
Статті
У відповідності з типовим шаблоном.
